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The ODIC phase of adamantane (208 K-541 K) was studied by Raman light scattering between 209 K and 500 K. The 1 220 cm-1, E symmetry, vibrational line was recorded with Eg and F2g symmetries. The Eg spectra, due to ordered molecules, are broadened by a residence time effect. The F2g spectra, which correspond to molecules as they rotate, could be attributed to the modification of the internal vibration by the environment during the molecular reorientations

Temperature dependence of internal bandwidths in plastic adamantane by Raman light scattering