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The energy transfer reaction between Ar(3P0), Ar( 3P2) and molecules of N2 was studied in the afterglow of a pulsed electrodeless discharge. The population decays of the metastable argon atoms and the intensity decays of the nitrogen second positive emission bands were monitored simultaneously. A dye laser was used to selectively depopulate each metastable argon species and the relative variations were checked on the intensity of the nitrogen second positive bands. Relative reaction rates in rotational and vibrational excitation of N2(C 3Πu) by Ar(3P0) and Ar( 3P2) were obtained

Relative reaction rates in rotational and vibrational excitation of N2(C 3Πu) by Ar*(3P0 ) and Ar*(3P2) metastable atoms

Relative reaction rates in rotational and vibrational excitation of N2(C 3Πu) by Ar(3P0 ) and Ar(3P2) metastable atoms