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A surface structure of submonolayer methanethiol CH3SH molecularly adsorbed on Cu(100) has been investigated by means of S K-edge SEXAFS and NEXAFS. From the analysis of these spectra, it was revealed that the CH3SH molecule adsorbs as a methanethiolate (CH3S-) with the S-C bond nearly perpendicular to the surface. SEXAFS has clarified that the S atom locates at the fourfold hollow site and the S-C and S-Cu bond distances are, respectively, 1.82±0.02 and 2.29±0.03 Å. Although it was reported that the adsorption of methanethiol induces surface reconstruction on the Cu(111) surface, we have observed neither reconstruction nor large strain ou the Cu(100) surface

Structure of CH3SH on Cu(100) Studied by S-K SEXAFS and NEXAFS

Structure of CH₃SH on Cu(100) Studied by S-K SEXAFS and NEXAFS