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We demonstrate a new method for multidimensional coherent spectroscopy of nanostructures. We use a heterodyne technique implemented with a confocal microscope to record the amplitude and phase of all degenerate third-order wave-mixing processes.

Vibrational Interferometry Enables Single-Scan Acquisition of all χ(3)Multi-Dimensional Coherent Spectra

Vibrational Interferometry Enables Single-Scan Acquisition of all χ⁽³⁾Multi-Dimensional Coherent Spectra