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Frequency upconversion of high-power visible or ultraviolet laser radiation by nonlinear optical processes in gases and metal vapors is a well established method to build coherent, high spectral brightness and tunable vacuum or extreme ultraviolet sources ("VUV" or "XUV" lasers).They provide a powerful tool for spectroscopy of atoms and small molecules through direct excitation of high lying electronic states such as Rydberg or valence states. Fundamental applications concern high resolution spectroscopy, molecular structure and molecular dynamics in the process of photodissocia tion or photoionizati on. Application fields are trace detection, plasma diagnostics, surface photochemistry.

annales de physique

Génération de rayonnement VUV et XUV cohérent par conversion de fréquence dans les gaz et les vapeurs métalliques. Utilisation en physique atomique et moléculaire