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A series of twelve two-coordinate coinage metal, Cu, Ag and Au, complexes with carbene-metal-amide structures were prepared and used to study the correlation of the overlap between the hole and electron NTOs with the electronic and photophysical properties of these TADF emitters.

journal of materials chemistry. c

Toward rational design of TADF two-coordinate coinage metal complexes: understanding the relationship between natural transition orbital overlap and photophysical properties