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Core–shell particles with a Prussian blue analogue Rb  a  Co  b  [Fe(CN) 6 ] c · m H 2 O core and different shell thicknesses are studied as the cores undergo both thermal and light-induced spin transitions, revealing different mechanisms for accommodating strain.

Interplay between core and shell in a RbCoFe@RbNiCo Prussian blue analogue spin transition heterostructure