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The electronic properties of molecular conductors are varied by substituting ions with extended wave functions to enlarge the bandwidth  W.  This enables them to cross the Mott insulator-to-metal phase transition by reducing electronic correlations  U / W .

journal of materials chemistry. c

Chemical tuning of molecular quantum materials κ-[(BEDT-TTF)1−x(BEDT-STF)x]2Cu2(CN)3: from the Mott-insulating quantum spin liquid to metallic Fermi liquid