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Bio-inspired [FeFe]-hydrogenase complexes and B(C 6 F 5 ) 3  form FLPs that are able to activate H 2 , providing rare examples of inverted enzymatic reactivity. The influence of the symmetry/asymmetry of coordination is studied  via  DFT.

chemical science

Geometrical influence on the non-biomimetic heterolytic splitting of H<sub>2</sub> by bio-inspired [FeFe]-hydrogenase complexes: a rare example of <i>inverted</i> frustrated Lewis pair based reactivity

Geometrical influence on the non-biomimetic heterolytic splitting of H2 by bio-inspired [FeFe]-hydrogenase complexes: a rare example of inverted frustrated Lewis pair based reactivity

Geometrical influence on the non-biomimetic heterolytic splitting of H₂ by bio-inspired [FeFe]-hydrogenase complexes: a rare example of inverted frustrated Lewis pair based reactivity