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An efficient hydrogen-bonding assisted directing strategy has been identified, which enables the Pd-catalyzed highly regioselective and diastereodivergent 3,4-difunctionalized aminomethylative annulation of dienyl alcohols with aminals.

chemical science

Highly Regioselective and Ligand-Controlled Diastereodivergent Aminomethylative Annulation of Dienyl Alcohols Enabled by Hydrogen-Bonding Assisting Effect