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The heterobimetallic actinide nitride [(NR 2 ) 3 U V (μ-N)Th IV (NR 2 ) 3 ] (R = SiMe 3 ) has an  m  J  = 5/2 ground state and its highest energy 5f excited state is primarily 5f-N nitride  σ-antibonding in character.

Synthesis of a heterobimetallic actinide nitride and an analysis of its bonding