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Co-crystallization of the cationic complex [Fe(3-bpp)2] 2+  with fractionally charged TCNQ  δ −  anions (0 &lt;  δ  &lt; 1) affords semiconducting spin-crossover (SCO) materials. The abruptness of SCO is strongly dependent on the interstitial solvent content.

chemical science

Optimization of crystal packing in semiconducting spin-crossover materials with fractionally charged TCNQδ− anions (0 &lt; δ &lt; 1)