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A novel salt-inclusion fluoroiodate nonlinear optical material, [GaF(H 2 O)][IO 3 F], is derived from CsIO 2 F 2  through polycation substitution, and it exhibits an intense SHG effect of 10 times that of KH 2 PO 4  and improved overall performance.

[GaF(H2O)][IO3F]: a promising NLO material obtained by anisotropic polycation substitution

[GaF(H₂O)][IO₃F]: a promising NLO material obtained by anisotropic polycation substitution