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Cibalackrot-type compounds are Hückel instead of Baird aromatic in their first triplet states (T 1 ). By choice of substituents and additional benzannelation we adjust the T 1  energies, providing a new strategy for singlet fission chromophore design.

Excited state character of Cibalackrot-type compounds interpreted in terms of Hückel-aromaticity: a rationale for singlet fission chromophore design