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Three-step method optimizes multilayer emulsion for maximum tannic acid (TA) amount at surfaces. (1) TA–emulsifier bulk interactions assessed. (2) LbL films built for optimal TA presence. (3) Emulsions built as per LbL design and TA action evaluated.

Towards the systematic design of multilayer O/W emulsions with tannic acid as an interfacial antioxidant