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A convenient design of pyrazolo[3,4- c ]pyrazoles is reported through hydrazine condensations and C–N Ullmann-type cross-coupling reactions. Chemoselective bromination followed by Suzuki–Miyaura cross-coupling reactions access to a variety of modulated heterobicycles.

Access and modulation of substituted 1-methyl-1,6-dihydropyrazolo[3,4-c]pyrazoles