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Two organic ionic crystals were successfully synthesized, namely [N(CH 2 CH 3 ) 3 (CH 2 Cl)][ClO 4 ] (1) and [N(CH 2 CH 3 ) 3 (CH 2 Cl)][BF 4 ] (2), with high-temperature reversible phase transitions. In addition, compounds 1 and 2 also show obvious CD signals.

Dielectric switching from a high temperature plastic phase transition in two organic salts with chiral features