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We present a dual passivation approach for p–i–n perovskite solar cells using phenethylammonium chloride that simultaneously passivates defects at the grain boundaries and the perovskite/C 60  interface, thus substantially enhancing both  V  OC  and FF.

Two birds with one stone: dual grain-boundary and interface passivation enables >22% efficient inverted methylammonium-free perovskite solar cells