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In the  operando  solar cell using Ruddlesden–Popper perovskite (RPP), we visualize an abnormal heterogeneity ranging from the lateral long-range to local sub-grain scale with a unitary 2D/3D hybrid, closely correlating to the charge-carrier dynamics.

Abnormal spatial heterogeneity governing the charge-carrier mechanism in efficient Ruddlesden–Popper perovskite solar cells