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Gallaphosphene 1 reacts with a series of polar X–H bonds exclusively with 1,2 addition to the Ga–P double bond. The gallium atom serve as electrophile whereas the nucleophilic phosphorous atom is protonated by the H-acidic substrates.

Selective 1,2 addition of polar X–H bonds to the Ga–P double bond of gallaphosphene L(Cl)GaPGaL