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A linear dependence of the lithium transference number and the composition of the polyester–polycarbonate copolymer electrolyte host material was discovered, and the coordination properties causing the trend were investigated with DFT calculations.

physical chemistry chemical physics/pccp. physical chemistry chemical physics

The role of coordination strength in solid polymer electrolytes: compositional dependence of transference numbers in the poly(ε-caprolactone)–poly(trimethylene carbonate) system