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Single-atom Ni terminating agent is introduced to coordinate with sp 2  or sp 3  N atoms in the heptazine units of PCN, realizing visible-light photocatalytic overall water splitting to H 2 O 2  and H 2  without additional cocatalyst.

chemical science

Single-atom nickel terminating sp<sup>2</sup> and sp<sup>3</sup> nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting

Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting

Single-atom nickel terminating sp² and sp³ nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting