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Several unique reactivity patterns of the Ni/JoSPOphos manifold, including facile hydrogen transfer  via  the two-step oxidative addition/migratory insertion and C(sp 2 )–H activation  via  an unconventional σ-CAM mechanism, were disclosed in this work.

Understanding the unique reactivity patterns of nickel/JoSPOphos manifold in the nickel-catalyzed enantioselective C–H cyclization of imidazoles