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We report the first thorium–cyclobutadienyl complex, a new type of heteroleptic actinocene, that exhibits ‘an alkene-like’ thorium–η 2 -cyclooctatetraenyl interaction.

Heteroleptic actinocenes: a thorium(iv)–cyclobutadienyl–cyclooctatetraenyl–di-potassium-cyclooctatetraenyl complex