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5-Amine-2-(4-amino-benzene)-1-phenyl-benzimidazole ( N -PhPABZ) was successfully synthesized and polymerized with 3,3',4,4'-biphenyl tetracarboxylic dianhydride (BPDA) to obtain a novel N -phenyl-poly(benzimidazole imide) ( N -Ph-PBII). The successful incorporation of N -phenyl addressed the issue of high H 2 O-absorption of traditional PBIIs while retained the superheat resistance property. The resulting N -Ph-PBII possessed a high glass-transition temperature ( T  g ) up to 425 °C and a low affinity for water of 1.4%. Furthermore, the loose molecular packing and noncoplanar structures led to an increase in optical transparency for the modified PBII.

Incorporation ofN-phenyl in poly(benzimidazole imide)s and improvement in H2O-absorbtion and transparency

Incorporation ofN-phenyl in poly(benzimidazole imide)s and improvement in H₂O-absorbtion and transparency