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A simple and efficient asymmetric synthesis of THBCs through a chiral thiosquaramide 11b catalyzed imine reduction of dihydro-β-carbolines ( 17a−f ) and syntheses of (−)-coerulescine and (–)-horsfiline via enantioselective oxidative rearrangement.

rsc advances

Bifunctional thiosquaramide catalyzed asymmetric reduction of dihydro-β-carbolines and enantioselective synthesis of (−)-coerulescine and (−)-horsfiline by oxidative rearrangement