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Two sets of Fe III/II  complexes, synthesized from  N , N ′-diisopropyl piperazine-2,3-dithione ( i Pr 2 Dt 0 ) and  N , N ′-dimethyl piperazine-2,3-dithione (Me 2 Dt 0 ) ligands, exhibit electronically asymmetrical ligands with metal–ligand orbital mixing.

Syntheses, spectroscopic, redox, and structural properties of homoleptic Iron(III/II) dithione complexes