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The first azadithiolato-bridged NiFe model complexes with a general formula [CpNi{(μ-SCH 2 ) 2 NR}Fe(CO)(diphos)]BF 4  have been synthesized, characterized, and for some of them found to be catalysts for proton reduction to H 2  under CV conditions.

rsc advances

Heterodinuclear nickel(<scp>ii</scp>)–iron(<scp>ii</scp>) azadithiolates as structural and functional models for the active site of [NiFe]-hydrogenases

Heterodinuclear nickel(ii)–iron(ii) azadithiolates as structural and functional models for the active site of [NiFe]-hydrogenases