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A solvent-controlled and heteroatom-dictated protocol for the transition metal-free addition of alkenyl Grignard reagents to lactam esters has been developed, leading to the chemo- and regioselective synthesis of lactam-tethered homoallylic ketones.

rsc advances

Transition metal-free domino acyl substitution/Michael addition of alkenyl Grignard reagents to lactam esters: synthesis of lactam-bearing homoallylic ketones