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A tetrafluoroaryl azide group attached to diphenylalanine  via  a carbamate linker provides a strong and stable hydrogel that undergoes a gel-to-solution transition following a rapid bioorthogonal 1,3,-dipolar cycloaddition.

Tetrafluoroaryl azide as an N-terminal capping group for click-to-dissolve diphenylalanine hydrogels