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Triarylamines are demonstrated as novel, tunable electroactivated photocatalysts that use dispersion precomplexation to harness the full potential of the visible photon (&gt;4.0 V  vs.  SCE) in anti-Kasha photo(electro)chemical super-oxidations of arenes.

Hole-mediated photoredox catalysis: tris(p-substituted)biarylaminium radical cations as tunable, precomplexing and potent photooxidants