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We report the design and synthesis of three  N -annulated perylene diimide (PDI) compounds containing sterically bulky alkyl-substituted benzyl moieties (PDI- X , where  X  = 1, 2, 3) and explore their use as light emitting materials in solution processed OLED devices.

Improved performance of solution processed OLEDs using N-annulated perylene diimide emitters with bulky side-chains