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Sequential embedding of metal complexes of 4′-(pyridin-4-yl)-2,2′:6′,2′′-terpyridine to a surface-enhanced supports pre-functionalized with a templating layer results in hetero-bimetallic (Os–Fe, Co–Fe) and hetero-trimetallic (Co–Os–Fe) monolayer materials.

Multiple electrochemically accessible colour states in surface-confined metal–organic monolayers: stepwise embedding of individual metal centres