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Ru-CNN(H) complexes are efficient precatalysts in the hydrogenation and dehydrogenation of N-heterocycles. Under basic conditions, these derivatives lead to the formation of Ru(0) species that are observed under catalytic conditions.

Hydrogenation/dehydrogenation of N-heterocycles catalyzed by ruthenium complexes based on multimodal proton-responsive CNN(H) pincer ligands