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The reactivity of [{Cp'''Fe(CO)2}2(μ,η1 : 1-P4)] (1) towards half-sandwich complexes of Ru(ii), Rh(iii), and Ir(iii) is studied. The coordination of these Lewis acids leads to a rearrangement of the P4 butterfly unit to form complexes with either an aromatic cyclo-P4R2 unit (R = Cp'''Fe(CO)2) or a catena-tetraphosphaene entity.

From a P4 butterfly scaffold to cyclo- and catena-P4 units

From a P₄ butterfly scaffold to cyclo- and catena-P₄ units