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Under a mild external pressure of 0.1 GPa valence tautomeric compounds {[Mn 2 (NITIm) 3 ]X} n  with nitronyl nitroxide radical NITIm and X = ClO 4  −  or BF 4  −  have their conversion shifted upwards by almost 40 K with respect to room temperature.

Hypersensitive pressure-dependence of the conversion temperature of hysteretic valence tautomeric manganese–nitronyl nitroxide radical 2D-frameworks