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A unique example of electroswitchable spin crossover molecular nanomagnet which proceeds through one-electron oxidation of the slow-relaxing paramagnetic low-spin Co II  ion ( S  Co  = 1/2, ON) to the diamagnetic low-spin Co III  ion ( S  Co  = 0, OFF).

chemical communications

Electroswitching of the single-molecule magnet behaviour in an octahedral spin crossover cobalt(<scp>ii</scp>) complex with a redox-active pyridinediimine ligand

Electroswitching of the single-molecule magnet behaviour in an octahedral spin crossover cobalt(ii) complex with a redox-active pyridinediimine ligand