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A unique chemoselectivity to base-promoted defluorinative and Cu-catalyzed aerobic oxidative non-defluorinative [5 + 1] cycloaddition of fluoride unsaturated ketones with ammonium salts was demonstrated.

chemical science

Controlled chemoselective defluorination and non-defluorination for [5 + 1] aromatic annulation <i>via</i> Meisenheimer-type nitrogen anion and radical intermediates

Controlled chemoselective defluorination and non-defluorination for [5 + 1] aromatic annulation via Meisenheimer-type nitrogen anion and radical intermediates