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Separation of TcO 4  –  by a cationic covalent organic framework is achieved for the first time, showing advantages of extremely fast sorption kinetics, ultrahigh uptake capacity, good anion-exchange selectivity, and excellent radiation resistance.

chemical science

Mechanism unravelling for ultrafast and selective 99TcO4− uptake by a radiation-resistant cationic covalent organic framework: a combined radiological experiment and molecular dynamics simulation study