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Melt shearing made the crystallinity of as-received PCL increased and the crystallization temperature raised by 7.7 °C. Polyvinyl acetals increased the spherulite size of PCL from a few microns to 200 μm and PVB improved the Young’s modulus of PCL by 67%.

Effect of polyvinyl acetals on non-isothermal crystallization behaviour and mechanical properties of poly(ε-caprolactone)