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We suggest a way to control the crystal orientation of LiFePO 4 using a magnetic field to obtain an advantageous structure for lithium ion conduction. We examined the magnetic properties of LiFePO 4 such as magnetism and magnetic susceptibility, which are closely related to the crystal rotation in an external magnetic field, and considered how to use these properties for desired crystal orientation; thus, we successfully fabricated the crystal-aligned LiFePO 4 , in which the b -axis was highly aligned perpendicular to the surface of a current collector. Considering the low lithium ion conductivity of LiFePO 4 inherently originated from its one-dimensional path for lithium ion diffusion, the crystal-aligned LiFePO 4 potentially facilitates favorable transport kinetics for lithium ions during the charge/discharge process in lithium ion batteries. The crystal-aligned LiFePO 4 should afford lower electrode polarization than pristine LiFePO 4 , and thus the former consistently exhibited higher reversible capacity than the latter.

Crystal alignment of a LiFePO4 cathode material for lithium ion batteries using its magnetic properties

Crystal alignment of a LiFePO₄ cathode material for lithium ion batteries using its magnetic properties