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The synthesis of a redox series of neodymium species bearing the redox active pyridine(diimine) ligand, MesPDIMe, is reported. Spectroscopic and structural characterization supports each compound has a Nd(iii) centre, with the MesPDIMe ligand existing in four oxidation states.

A reduction series of neodymium supported by pyridine(diimine) ligands