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Single and double dearomatization of pyridine rings was observed in Mn I complexes with an N2S2 pyridinophane ligand via deprotonation of one or two CH 2 arms, respectively. In contrast to other N,S-donor pincer-like systems, the dearomatized (N2S2)Mn species were found to be stable, with the dearomatization being reversible.

Facile and reversible double dearomatization of pyridines in non-phosphine MnI complexes with N,S-donor pyridinophane ligand

Facile and reversible double dearomatization of pyridines in non-phosphine Mn^I complexes with N,S-donor pyridinophane ligand