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The synergism of the electronic properties of nickel and cobalt enables bimetallic NiCo complexes to process H 2 . The nickel-cobalt hydride [(dppe)Ni(pdt)(H)CoCp*] + ( [1H] +  ) arising from protonation of the reduced state 1 was found to be an efficient electrocatalyst for H 2 evolution with Cl 2 CHCOOH, and the oxidized [Ni(ii)Co(iii)] 2+ form is capable of activating H 2 to produce [1H] +  . The features of stereodynamics, acid-base properties, redox chemistry and reactivity of these bimetallic NiCo complexes in processing H 2 are potentially related to the active site of [NiFe]-H 2 ases.

Bimetallic nickel–cobalt hydrides in H2 activation and catalytic proton reduction

Bimetallic nickel–cobalt hydrides in H₂ activation and catalytic proton reduction