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A series of cationic complexes involving a pnictogen(iii) (Pn = P, As, Sb) centre and the tetradentate ligand tris((1-ethyl-benzoimidazol-2-yl)methyl)amine (BIMEt 3 ) have been synthesized and comprehensively characterized. Oxidation of [P(BIMEt 3 )] 3+ with XeF 2 provides access to [PF 2 (BIMEt 3 )] 3+ representing the first structurally characterized example of a phosphorus(v) centred trication.

chemical science

Tris(benzoimidazol)amine (L) complexes of pnictogen(<scp>iii</scp>) and pnictogen(<scp>v</scp>) cations and assessment of the [LP]3+/[LPF2]3+ redox couple

Tris(benzoimidazol)amine (L) complexes of pnictogen(iii) and pnictogen(v) cations and assessment of the [LP]3+/[LPF2]3+ redox couple

Tris(benzoimidazol)amine (L) complexes of pnictogen(iii) and pnictogen(v) cations and assessment of the [LP]³⁺/[LPF₂]³⁺ redox couple