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We describe the synthesis of electron acceptors consisting of bithiazolidinylidene (BT) derivatives incorporated into solution processible polymers. Novel BT-containing polymers displayed p-doping behavior when in contact with the n-type transition metal dichalcogenide (TMDC) MoS 2 . A work function (WF) increase of MoS 2 , resulting from contact with BT polymers, was measured by Kelvin probe force microscopy (KPFM), representing the first example of polymer p-doping of MoS 2 , which is beneficial for advancing the design of electronically tailored TMDCs.

Bithiazolidinylidene polymers: synthesis and electronic interactions with transition metal dichalcogenides