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Four anti-perovskite-type compounds, ZnNNi3, ZnCNi3, SnNCo3, and SnCCo3, aresynthesised through reactions between ingredient metal oxides and organiccompound melamine (C3H6N6). ZnNNi3 and ZnCNi3 are selectively synthesised bychoosing different reaction temperatures and nominal oxide-to-melamine ratios.SnNCo3 is synthesised for the first time by this melamine method. Resistivity,magnetisation, and heat capacity measurements reveal that SnNCo3 is acorrelated metal with a high density of states at the Fermi level. Our resultsdemonstrate that this feasible synthetic route using melamine is useful in thesearch for complex metal carbides and nitrides toward novel functionalmaterials.

Synthesis of anti-perovskite-type carbides and nitrides from metal oxides and melamine