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We present a combined experimental and theoretical study of state-to-state inelastic scattering of ND 3 (j = 1 1  - ) with D 2 (j = 0, 1, 2, 3) molecules at collision energies around 800 cm -1 . Using a crossed molecular beam apparatus which employs the combination of Stark deceleration and velocity map imaging, we observe the correlated rotational excitations of both collision partners. For D 2 , both elastic (Δj D 2  = 0), inelastic excitation (j = 0 →j = 2) and inelastic de-excitation (j = 2 →j = 0) processes are observed. For a number of final ND 3 states, inelastic channels in which D 2 is rotationally excited or de-excited appear surprisingly strong. The experimental results are in excellent agreement with the predictions from quantum scattering calculations which are based on an ab initio ND 3 -D 2 potential energy surface.

Direct observation of product-pair correlations in rotationally inelastic collisions of ND3 with D2

Direct observation of product-pair correlations in rotationally inelastic collisions of ND₃ with D₂