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The radiative cooling of highly excited carbon cluster cations of sizes N = 8, 10, 13-16 has been studied in an electrostatic storage ring. The cooling rate constants vary with cluster size from a maximum at N = 8 of 2.6 × 10 4 s -1 and a minimum at N = 13 of 4.4 × 10 3 s -1 . The high rates indicate that photon emission takes place from electronically excited ions, providing a strong stabilizing cooling of the molecules.

Radiative cooling of cationic carbon clusters, CN+, N = 8, 10, 13–16

Radiative cooling of cationic carbon clusters, C_N⁺, N = 8, 10, 13–16