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A new octacyanotungstate(v) based single chain magnet {[(Tpm)Co(DMF)W(CN) 8 ] 2 [Co(DMF) 4 ]·2DMF}  n  ( 1 , Tpm = 1,1,1-trispyrazoylmethane), with an effective barrier of 39.7(3) cm -1 is reported. The Ising-like magnetic anisotropy of the chain originates from the nearly parallel local orientations of the Co(ii) ions with the source of the uniaxial magnetic anisotropy being a trigonal distortion of the octahedral environment with the fac -tridentate capping Tpm ligand.

chemical science

Enforcing Ising-like magnetic anisotropy <i>via</i> trigonal distortion in the design of a W(<scp>v</scp>)–Co(<scp>ii</scp>) cyanide single-chain magnet

Enforcing Ising-like magnetic anisotropy via trigonal distortion in the design of a W(v)–Co(ii) cyanide single-chain magnet